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Signature analysis of single molecules using their noise signals

Date:
July 12, 2017
Source:
Osaka University
Summary:
Unique noise signatures have been obtained from single molecules interacting with carbon nanotube-based electronic devices.
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Noise is low-frequency random fluctuation that occurs in many systems, including electronics, environments, and organisms. Noise can obscure signals, so it is often removed from electronics and radio transmissions. The origin of noise in nanoscale electronics is currently of much interest, and devices that operate using noise have been proposed. Materials with a high surface-to-volume ratio are attractive for studying the noise produced by nanoscale electronics because they are very sensitive to changes of their surfaces. A representative material of this type is carbon nanotubes, which are rolled sheets of the graphene hexagonal network, which is only one carbon atom thick.

A Japanese collaboration led by Osaka University has explored the ability of single molecules to affect the noise generated by carbon nanotube-based nanoscale electronic devices. The team fabricated simple devices consisting of a carbon nanotube bridging two electrodes. The devices were exposed to different large molecules, causing some to bind to the carbon nanotube surface. It was found that different molecules gave unique noise signals related to the properties of the molecules. The strength of the interaction between the carbon nanotubes and molecules was able to be predicted from the obtained noise signals.

"The signal generated by the carbon nanotube device changed following the adsorption of specific single molecules," says first author Agung Setiadi. "This is because the adsorbed molecule generated a trap state in the carbon nanotube, which changed its conductance."

What this means is that the carbon nanotube-based devices were so sensitive that the researchers were able to detect unique signature from single molecules. The ability to characterize single molecules using highly sensitive nanoelectronics is an exciting prospect in the field of sensors, particularly for neuro- and biosensor applications.

"Use of noise signals to identify molecular activity ((interaction) or (active orbital)) is attractive for developing advanced sensing devices," explains corresponding author Megumi Akai-Kasaya. "We demonstrated that noise can be exploited to improve the signal detection ability of a device." The results of this successful demonstration will be published in the near future in a follow-up article.

Signal detection sensitivity may be increased through controllable noise generation. These carbon nanotube-based devices illustrate that it is possible to detect single molecules through their unique noise signatures in the device current signals. Improved knowledge of the molecular-level origin of noise should lead to the development of electronics that use noise to improve their performance rather than degrade it.


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Materials provided by Osaka University. Note: Content may be edited for style and length.


Journal Reference:

  1. Agung Setiadi, Hayato Fujii, Seiya Kasai, Ken-ichi Yamashita, Takuji Ogawa, Takashi Ikuta, Yasushi Kanai, Kazuhiko Matsumoto, Yuji Kuwahara, Megumi Akai-Kasaya. Room-temperature discrete-charge-fluctuation dynamics of a single molecule adsorbed on a carbon nanotube. Nanoscale, 2017; DOI: 10.1039/c7nr02534c

Cite This Page:

Osaka University. "Signature analysis of single molecules using their noise signals." ScienceDaily. ScienceDaily, 12 July 2017. <www.sciencedaily.com/releases/2017/07/170712110430.htm>.
Osaka University. (2017, July 12). Signature analysis of single molecules using their noise signals. ScienceDaily. Retrieved March 27, 2024 from www.sciencedaily.com/releases/2017/07/170712110430.htm
Osaka University. "Signature analysis of single molecules using their noise signals." ScienceDaily. www.sciencedaily.com/releases/2017/07/170712110430.htm (accessed March 27, 2024).

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