Manipulating nanoscale light in nanocavity of scanning tunneling microscope junctions

A research team at the Fritz-Haber Institute in Berlin, headed by Dr. Takashi Kumagai, now demonstrated that manipulation of nanolight spectrum can be attained by shaping accurately plasmonic gold tips with a focused ion beam (FIB) milling technique. As an exemplary demonstration, they produced a very sharp tip with a single groove on its shaft as shown in the scanning electron microscope picture. The spectral response of nanolight confined in the nanocavity formed by the grooved tip and an atomically flat silver surface was investigated by using STL that is the combination of electronic and optical spectroscopies using scanning tunneling microscopy. The STML spectra with the grooved tips exhibit a characteristic modulation resulting from Fabry-Pérot type interference of surface plasmon polaritons (SPPs) on the tip shaft as the standing wave formation is visualized in the electrodynamic simulation. The spectral modulation can be precisely controlled by the groove position on the shaft. They also demonstrated that the SPP Fabry-Pérot interference can be improved by optimizing the overall tip shape.

This work shows a great potential of the combination of scanning probe techniques and nano-fabrication of plasmonic tips using FIB in order to study the nature of nanolight and light-matter interactions in nanocavities, which are an important frontier of plasmonics and nanooptics. In addition, the FIB-fabricated plasmonic tips are generally applicable to s-SNOM techniques, thus paving the way for nanoscale imaging and spectroscopy with a high degree of accuracy. Moreover, spectral control of the intense near-field at the apex of plasmonic tips may open up new opportunities for the realization of coherent laser-triggered electron point sources for low-energy electron microscopy and holography techniques.